Huh. Shows I'm not keeping up with the game like I used to. I didn't know that external I2S connections had become a thing in the industry. When I worked (90s-early 2010s), it was an internal audio interface only (between chips on a board, not between two products).
A little bit of Googling tells me it was pushed by PS Audio as superior to SPDIF. Color me skeptical of that claim.
But what you describe seems nearly impossible. "More definition, detail retrieval, a blacker background, more "pop" to the music, more space between the instruments, clearer sound, etc." defies all my understanding of a digital audio interface. Even if one cable was totally defective, those differences are not what one would get. Instead there would be dropouts or no audio at all. What you describe are more analog effects, not something that can change in a digital interface.
Of course, you won't like my response, but your observations contradict conventional wisdom in digital audio and therefore, as the saying goes, extraordinary claims require extraordinary evidence.