I've always had mine crossed over at 80Hz. While I get what the graph is representing, I tried 120Hz, 100Hz, and 80Hz this evening and the 80Hz still sounded best to my ears. My listening environment is 9.1 and I was listening to multi-channel music as a test case. The bass just seemed fuller. I'm guessing because the 100Hz to 80Hz sound was coming from all around instead of just the sub. Maybe the dynamics of the room, I don't know.
However, the graph above is just for the S-150. I also have four SS-200's as side and back speakers in the mix. There was a time in my old setup with a Marantz receiver that Audyssey set my S-150's to 80Hz and my SS-200's to 60Hz. I didn't figure it out right away until I listened to the Eagles Hotel California Blu-ray Audio that seemed bass heavy in the surrounds and the bass was definitely being overdriven in my side and rear speakers. That is when I discovered the 60Hz crossover settings. When I put it back to 80Hz and played it again all was fine. I only bring this up because maybe I should try the S-150's at 100Hz and the SS-200s at 80Hz. Maybe Audyssey was telling me something about the SS-200s.
When I bought these speakers back in 2004, I knew the SS-150s were the natural match for the S-150's and the SS-250's for the S-250. Somewhere in the middle was the odd duck SS-200. The SS-200s had the larger woofer and two speakers on each side vs. the one per side in the SS-150's. For movies I'm sure the SS-150's would have been fine, but for multi-channel music I thought the SS-200's would be a better match.
I wonder how the SS-200's would graph?