Genelec 8351B (one speaker have max 113dB so for pair will be 116dB) is much more powerfull, than Genelec 7360A (109dB). So very low crossover frequency could be optimal. Hard to tell how low.Still tempted to drop the crossover to 50Hz. These 8351B's are SO GOOD already that it's barely different with or without the sub dialled in.
Genelec GLM doing everything automatically. If You want boost bass after calibration, use "Sound Character Profiler":Of note, I think I need to adjust the gain on the sub a little to compensate as you mention your sensitivity of both mains is higher than the single sub. Would GLM account for this or would I have to manually account for this myself?
... but remember - Genelec 7360A is very not optimal for Genelec 8351B, and after bass boost, 7360A will be ... more not optimal