Well, maybe. Or, maybe not.
A couple things you may not have realized or just don’t know (which is OK).
Group delay is not a constant. It changes with frequency and usually increases with decreasing frequency with subs. It’s expressed in milliseconds so you’re good there as far as how you’re going about it. The lower the crossover point, the greater the delay you’ll need to have a hopefully ideal transition between the subs and mains.
Not knowing the actual group delay and having no instrumentation, using your ears to obtain a smooth crossover is valid.
If it sounds good, go with it.
If you can run room correction software at some point in the future, you’ll want to remove the delay.
Factoid: at 70F degrees, the speed of sound is a hair over 13 inches per millisecond. Your delay is equivalent to moving your mains 9ft back from the listening position.
26 years ago, I couldn’t really get smooth in-room response from my two subs when they were by the mains. The area behind the speakers was huge and the room wasn’t perfectly regular. The bass modes were killer.
Doing a little research, it seemed that I should try leaving the right sub by the right main and move the left sub to the left rear corner.
Running the subs in mono and adjusting for corner gain from the rear sub helped a bit, but the listening position still suffered from some room modes. I delayed the rear sub and 11ms was the value that worked the best. While not perfect, it worked very well.
My system was a vintage Marantz pre driving the best active speakers Paradigm ever made (LCR-450’s). The subs were their Servo 15 model. The mains had 80Hz crossovers built in. I used a Digitech DSP-256 studio multi-effects processor to drive the subs and create surround sound.
I used my acquired knowledge and my ears to dial in better sound.